Fast fabrication of high entropy oxides electrodes for flexible zinc-ion batteries with high electrochemical performance

Research Article
Open access

Fast fabrication of high entropy oxides electrodes for flexible zinc-ion batteries with high electrochemical performance

Yuqi Nie 1*
  • 1 Southwest University    
  • *corresponding author 631607010324@mails.cqjtu.edu.cn
Published on 7 November 2023 | https://doi.org/10.54254/2755-2721/24/20230698
ACE Vol.24
ISSN (Print): 2755-273X
ISSN (Online): 2755-2721
ISBN (Print): 978-1-83558-069-1
ISBN (Online): 978-1-83558-070-7

Abstract

The expanding world population, increasing energy demand, and looming climate change urge the development of a sustainable energy future while safeguarding our vulnerable environment. To build a new flexible battery system, high entropy oxides are used as electrodes based on zinc-ion batteries. The battery system with the best electrochemical performance can be determined by a series of experimental designs. Here in I propose to develop a HEO electrode using a fast and clean laser deposition method. A series of tests are designed to verify the degree of performance improvement. In the further research planning, the electrode material can be produced with a metal removed from the HEOs alone and using the same synthetic method and performance measurements to determine the roles of each metal in the HEOs. Additionally, the anions in the HEOs can also be varied to study the impact of various anions on the cell's electrochemical performance. Finally, the particle size of the HEOs can be varied to establish a correspondence between particle size and electrochemical performance to facilitate the selection of the optimum particle sizes. The experimental results can further provide a theoretical basis for the commercial application of zinc-ion batteries in flexible power systems.

Keywords:

zinc-ion batteries, high entropy oxides, electrochemical performance, high energy and power density

Nie,Y. (2023). Fast fabrication of high entropy oxides electrodes for flexible zinc-ion batteries with high electrochemical performance. Applied and Computational Engineering,24,152-157.
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References

[1]. Selvakumaran D., Pan A. Q., Liang S. Q., et al. A review on recent developments and challenges of cathode materials for rechargeable aqueous Zn-ion batteries. JOURNAL OF MATERIALS CHEMISTRY A (2019), 7(31): 18209-18236.

[2]. Ming Jun, Guo Jing, Xia Chuan, et al. Zinc-ion batteries: Materials, mechanisms, and applications. Materials Science and Engineering: R: Reports (2019), 135: 58-84.

[3]. Li Ming, Li Zengqing, Ye Xiaorui, et al. Tendril-Inspired 900% Ultrastretching Fiber-Based Zn-Ion Batteries for Wearable Energy Textiles. ACS Applied Materials & Interfaces (2021), 13(14): 17110-17117.

[4]. Zhang Y., Wang Q. R., Bi S. S., et al. Flexible all-in-one zinc-ion batteries. NANOSCALE (2019), 11(38): 17630-17636.

[5]. Xu Zhixiao, Li Matthew, Sun Wenyuan, et al. An Ultrafast, Durable, and High-Loading Polymer Anode for Aqueous Zinc-Ion Batteries and Supercapacitors. Advanced Materials (2022), 34(23): 2200077.

[6]. Zhang Ning, Chen Xuyong, Yu Meng, et al. Materials chemistry for rechargeable zinc-ion batteries. CHEMICAL SOCIETY REVIEWS (2020), 49(13): 4203-4219.

[7]. Zhu Kaiyue, Wu Tao, Sun Shichen, et al. Electrode Materials for Practical Rechargeable Aqueous Zn-Ion Batteries: Challenges and Opportunities. ChemElectroChem (2020), 7(13): 2714-2734.

[8]. Nguyen Thi Xuyen, Patra Jagabandhu, Chang Jeng-Kuei, et al. High entropy spinel oxide nanoparticles for superior lithiation–delithiation performance. Journal of Materials Chemistry A (2020), 8(36): 18963-18973.

[9]. Wang Dan, Jiang Shunda, Duan Chanqin, et al. Spinel-structured high entropy oxide (FeCoNiCrMn)3O4 as anode towards superior lithium storage performance. Journal of Alloys and Compounds (2020), 844: 156158.

[10]. Wang Q. S., Sarkar A., Wang D., et al. Multi-anionic and -cationic compounds: new high entropy materials for advanced Li-ion batteries. ENERGY & ENVIRONMENTAL SCIENCE (2019), 12(8).

[11]. Wang Bing, Wang Cheng, Yu Xiwen, et al. General synthesis of high-entropy alloy and ceramic nanoparticles in nanoseconds. Nature Synthesis (2022), 1(2): 138-146.

[12]. Koczkur Kallum M., Mourdikoudis Stefanos, Polavarapu Lakshminarayana, et al. Polyvinylpyrrolidone (PVP) in nanoparticle synthesis. Dalton Transactions (2015), 44(41): 17883-17905.

[13]. Bischoff Christian, Fitz Oliver, Schiller Christian, et al. Investigating the Impact of Particle Size on the Performance and Internal Resistance of Aqueous Zinc Ion Batteries with a Manganese Sesquioxide Cathode, Batteries(2018).

[14]. Bläubaum Lars, Röder Fridolin, Nowak Christine, et al. Impact of Particle Size Distribution on Performance of Lithium-Ion Batteries [J]. ChemElectroChem, 2020, 7(23): 4755-4766.

Cite this article

Nie,Y. (2023). Fast fabrication of high entropy oxides electrodes for flexible zinc-ion batteries with high electrochemical performance. Applied and Computational Engineering,24,152-157.

Data availability

The datasets used and/or analyzed during the current study will be available from the authors upon reasonable request.

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About volume

Volume title: Proceedings of the 2023 International Conference on Functional Materials and Civil Engineering

ISBN：978-1-83558-069-1(Print) / 978-1-83558-070-7(Online)
Editor：Bhupesh Kumar
Conference website: https://www.conffmce.org/
Conference date: 26 August 2023
Series: Applied and Computational Engineering
Volume number: Vol.24
ISSN：2755-2721(Print) / 2755-273X(Online)

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References

[1]. Selvakumaran D., Pan A. Q., Liang S. Q., et al. A review on recent developments and challenges of cathode materials for rechargeable aqueous Zn-ion batteries. JOURNAL OF MATERIALS CHEMISTRY A (2019), 7(31): 18209-18236.

[2]. Ming Jun, Guo Jing, Xia Chuan, et al. Zinc-ion batteries: Materials, mechanisms, and applications. Materials Science and Engineering: R: Reports (2019), 135: 58-84.

[3]. Li Ming, Li Zengqing, Ye Xiaorui, et al. Tendril-Inspired 900% Ultrastretching Fiber-Based Zn-Ion Batteries for Wearable Energy Textiles. ACS Applied Materials & Interfaces (2021), 13(14): 17110-17117.

[4]. Zhang Y., Wang Q. R., Bi S. S., et al. Flexible all-in-one zinc-ion batteries. NANOSCALE (2019), 11(38): 17630-17636.

[5]. Xu Zhixiao, Li Matthew, Sun Wenyuan, et al. An Ultrafast, Durable, and High-Loading Polymer Anode for Aqueous Zinc-Ion Batteries and Supercapacitors. Advanced Materials (2022), 34(23): 2200077.

[6]. Zhang Ning, Chen Xuyong, Yu Meng, et al. Materials chemistry for rechargeable zinc-ion batteries. CHEMICAL SOCIETY REVIEWS (2020), 49(13): 4203-4219.

[7]. Zhu Kaiyue, Wu Tao, Sun Shichen, et al. Electrode Materials for Practical Rechargeable Aqueous Zn-Ion Batteries: Challenges and Opportunities. ChemElectroChem (2020), 7(13): 2714-2734.

[8]. Nguyen Thi Xuyen, Patra Jagabandhu, Chang Jeng-Kuei, et al. High entropy spinel oxide nanoparticles for superior lithiation–delithiation performance. Journal of Materials Chemistry A (2020), 8(36): 18963-18973.

[9]. Wang Dan, Jiang Shunda, Duan Chanqin, et al. Spinel-structured high entropy oxide (FeCoNiCrMn)3O4 as anode towards superior lithium storage performance. Journal of Alloys and Compounds (2020), 844: 156158.

[10]. Wang Q. S., Sarkar A., Wang D., et al. Multi-anionic and -cationic compounds: new high entropy materials for advanced Li-ion batteries. ENERGY & ENVIRONMENTAL SCIENCE (2019), 12(8).

[11]. Wang Bing, Wang Cheng, Yu Xiwen, et al. General synthesis of high-entropy alloy and ceramic nanoparticles in nanoseconds. Nature Synthesis (2022), 1(2): 138-146.

[12]. Koczkur Kallum M., Mourdikoudis Stefanos, Polavarapu Lakshminarayana, et al. Polyvinylpyrrolidone (PVP) in nanoparticle synthesis. Dalton Transactions (2015), 44(41): 17883-17905.

[13]. Bischoff Christian, Fitz Oliver, Schiller Christian, et al. Investigating the Impact of Particle Size on the Performance and Internal Resistance of Aqueous Zinc Ion Batteries with a Manganese Sesquioxide Cathode, Batteries(2018).

[14]. Bläubaum Lars, Röder Fridolin, Nowak Christine, et al. Impact of Particle Size Distribution on Performance of Lithium-Ion Batteries [J]. ChemElectroChem, 2020, 7(23): 4755-4766.

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